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Electrochemical control of [FeFe]-hydrogenase single crystals reveals complex redox populations at the catalytic site
Elucidating the distribution of intermediates at the active site of redox metalloenzymes is vital to understanding their highly efficient catalysis. Here we demonstrate that it is possible to generate, and detect, the key catalytic redox states of an [FeFe]-hydrogenase in a protein crystal. Individu...
| Autores principales: | , , , , , |
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| Formato: | Online Artículo Texto |
| Lenguaje: | English |
| Publicado: |
The Royal Society of Chemistry
2021
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| Materias: | |
| Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8453692/ https://www.ncbi.nlm.nih.gov/pubmed/34545877 http://dx.doi.org/10.1039/d1dt02219a |