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Direct Evidence on the Mechanism of Methane Conversion under Non‐oxidative Conditions over Iron‐modified Silica: The Role of Propargyl Radicals Unveiled
Radical‐mediated gas‐phase reactions play an important role in the conversion of methane under non‐oxidative conditions into olefins and aromatics over iron‐modified silica catalysts. Herein, we use operando photoelectron photoion coincidence spectroscopy to disentangle the elusive C(2+) radical int...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
John Wiley and Sons Inc.
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8596584/ https://www.ncbi.nlm.nih.gov/pubmed/34459534 http://dx.doi.org/10.1002/anie.202107553 |