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Stripping away ion hydration shells in electrical double-layer formation: Water networks matter

The double layer at the solid/electrolyte interface is a key concept in electrochemistry. Here, we present an experimental study combined with simulations, which provides a molecular picture of the double-layer formation under applied voltage. By THz spectroscopy we are able to follow the stripping...

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Detalles Bibliográficos
Autores principales: Alfarano, Serena R., Pezzotti, Simone, Stein, Christopher J., Lin, Zhou, Sebastiani, Federico, Funke, Sarah, Hoberg, Claudius, Kolling, Inga, Ma, Chun Yu, Mauelshagen, Katja, Ockelmann, Thorsten, Schwaab, Gerhard, Fu, Li, Brubach, Jean-Blaise, Roy, Pascale, Head-Gordon, Martin, Tschulik, Kristina, Gaigeot, Marie-Pierre, Havenith, Martina
Formato: Online Artículo Texto
Lenguaje:English
Publicado: National Academy of Sciences 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8617503/
https://www.ncbi.nlm.nih.gov/pubmed/34782461
http://dx.doi.org/10.1073/pnas.2108568118