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Electrostatic Discovery Atomic Force Microscopy
[Image: see text] While offering high resolution atomic and electronic structure, scanning probe microscopy techniques have found greater challenges in providing reliable electrostatic characterization on the same scale. In this work, we offer electrostatic discovery atomic force microscopy, a machi...
Autores principales: | , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2021
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8793147/ https://www.ncbi.nlm.nih.gov/pubmed/34806866 http://dx.doi.org/10.1021/acsnano.1c06840 |
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author | Oinonen, Niko Xu, Chen Alldritt, Benjamin Canova, Filippo Federici Urtev, Fedor Cai, Shuning Krejčí, Ondřej Kannala, Juho Liljeroth, Peter Foster, Adam S. |
author_facet | Oinonen, Niko Xu, Chen Alldritt, Benjamin Canova, Filippo Federici Urtev, Fedor Cai, Shuning Krejčí, Ondřej Kannala, Juho Liljeroth, Peter Foster, Adam S. |
author_sort | Oinonen, Niko |
collection | PubMed |
description | [Image: see text] While offering high resolution atomic and electronic structure, scanning probe microscopy techniques have found greater challenges in providing reliable electrostatic characterization on the same scale. In this work, we offer electrostatic discovery atomic force microscopy, a machine learning based method which provides immediate maps of the electrostatic potential directly from atomic force microscopy images with functionalized tips. We apply this to characterize the electrostatic properties of a variety of molecular systems and compare directly to reference simulations, demonstrating good agreement. This approach offers reliable atomic scale electrostatic maps on any system with minimal computational overhead. |
format | Online Article Text |
id | pubmed-8793147 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-87931472022-01-28 Electrostatic Discovery Atomic Force Microscopy Oinonen, Niko Xu, Chen Alldritt, Benjamin Canova, Filippo Federici Urtev, Fedor Cai, Shuning Krejčí, Ondřej Kannala, Juho Liljeroth, Peter Foster, Adam S. ACS Nano [Image: see text] While offering high resolution atomic and electronic structure, scanning probe microscopy techniques have found greater challenges in providing reliable electrostatic characterization on the same scale. In this work, we offer electrostatic discovery atomic force microscopy, a machine learning based method which provides immediate maps of the electrostatic potential directly from atomic force microscopy images with functionalized tips. We apply this to characterize the electrostatic properties of a variety of molecular systems and compare directly to reference simulations, demonstrating good agreement. This approach offers reliable atomic scale electrostatic maps on any system with minimal computational overhead. American Chemical Society 2021-11-22 2022-01-25 /pmc/articles/PMC8793147/ /pubmed/34806866 http://dx.doi.org/10.1021/acsnano.1c06840 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Oinonen, Niko Xu, Chen Alldritt, Benjamin Canova, Filippo Federici Urtev, Fedor Cai, Shuning Krejčí, Ondřej Kannala, Juho Liljeroth, Peter Foster, Adam S. Electrostatic Discovery Atomic Force Microscopy |
title | Electrostatic
Discovery Atomic Force Microscopy |
title_full | Electrostatic
Discovery Atomic Force Microscopy |
title_fullStr | Electrostatic
Discovery Atomic Force Microscopy |
title_full_unstemmed | Electrostatic
Discovery Atomic Force Microscopy |
title_short | Electrostatic
Discovery Atomic Force Microscopy |
title_sort | electrostatic
discovery atomic force microscopy |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8793147/ https://www.ncbi.nlm.nih.gov/pubmed/34806866 http://dx.doi.org/10.1021/acsnano.1c06840 |
work_keys_str_mv | AT oinonenniko electrostaticdiscoveryatomicforcemicroscopy AT xuchen electrostaticdiscoveryatomicforcemicroscopy AT alldrittbenjamin electrostaticdiscoveryatomicforcemicroscopy AT canovafilippofederici electrostaticdiscoveryatomicforcemicroscopy AT urtevfedor electrostaticdiscoveryatomicforcemicroscopy AT caishuning electrostaticdiscoveryatomicforcemicroscopy AT krejciondrej electrostaticdiscoveryatomicforcemicroscopy AT kannalajuho electrostaticdiscoveryatomicforcemicroscopy AT liljerothpeter electrostaticdiscoveryatomicforcemicroscopy AT fosteradams electrostaticdiscoveryatomicforcemicroscopy |