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Picosecond pulse-shaping for strong three-dimensional field-free alignment of generic asymmetric-top molecules

Fixing molecules in space is a crucial step for the imaging of molecular structure and dynamics. Here, we demonstrate three-dimensional (3D) field-free alignment of the prototypical asymmetric top molecule indole using elliptically polarized, shaped, off-resonant laser pulses. A truncated laser puls...

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Detalles Bibliográficos
Autores principales: Mullins, Terry, Karamatskos, Evangelos T., Wiese, Joss, Onvlee, Jolijn, Rouzée, Arnaud, Yachmenev, Andrey, Trippel, Sebastian, Küpper, Jochen
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8931173/
https://www.ncbi.nlm.nih.gov/pubmed/35301292
http://dx.doi.org/10.1038/s41467-022-28951-z