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Electronic coherences in nonadiabatic molecular photophysics revealed by time-resolved photoelectron spectroscopy

Time-resolved photoelectron spectroscopy (TRPES) signals that monitor the relaxation of the RNA base uracil upon optical excitation are simulated. Distinguishable signatures of coherence dynamics at conical intersections are identified, with temporal and spectral resolutions determined by the durati...

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Detalles Bibliográficos
Autores principales: Cavaletto, Stefano M., Keefer, Daniel, Mukamel, Shaul
Formato: Online Artículo Texto
Lenguaje:English
Publicado: National Academy of Sciences 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8931378/
https://www.ncbi.nlm.nih.gov/pubmed/35254910
http://dx.doi.org/10.1073/pnas.2121383119