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To unravel the connection between the non-equilibrium and equilibrium solvation dynamics of tryptophan: success and failure of the linear response theory of fluorescence Stokes shift
The connections between the non-equilibrium solvation dynamics upon optical transitions and the system's equilibrium fluctuations are explored in aqueous liquid. Linear response theory correlates time-dependent fluorescence with the equilibrium time correlation functions. In the previous work [...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9053704/ https://www.ncbi.nlm.nih.gov/pubmed/35517244 http://dx.doi.org/10.1039/d0ra01227k |