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Electronic structure analysis of electrochemical CO(2) reduction by iron-porphyrins reveals basic requirements for design of catalysts bearing non-innocent ligands

Electrocatalytic CO(2) reduction is a possible solution to the increasing CO(2) concentration in the earth’s atmosphere, because it enables storage of energy while using the harmful CO(2) feedstock as a starting material. Notably, iron(ii) tetraphenylporphyrin, [Fe(II)(TPP)](0) (TPP(2−) = tetrapheny...

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Detalles Bibliográficos
Autores principales: Tarrago, Maxime, Ye, Shengfa, Neese, Frank
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9430493/
https://www.ncbi.nlm.nih.gov/pubmed/36128248
http://dx.doi.org/10.1039/d2sc01863b