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Using symmetry to control viscoelastic waves in pillar arrays

Solutions of macromolecules exhibit viscoelastic properties and unlike Newtonian fluids, they may break time-reversal symmetry at low Reynolds numbers resulting in elastic turbulence. Furthermore, under some conditions, instead of the chaotic turbulence, the result is large-scale waves in the form o...

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Autores principales: Beech, Jason P., Ström, Oskar E., Turato, Enrico, Tegenfeldt, Jonas O.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10603618/
https://www.ncbi.nlm.nih.gov/pubmed/37901264
http://dx.doi.org/10.1039/d3ra06565k
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author Beech, Jason P.
Ström, Oskar E.
Turato, Enrico
Tegenfeldt, Jonas O.
author_facet Beech, Jason P.
Ström, Oskar E.
Turato, Enrico
Tegenfeldt, Jonas O.
author_sort Beech, Jason P.
collection PubMed
description Solutions of macromolecules exhibit viscoelastic properties and unlike Newtonian fluids, they may break time-reversal symmetry at low Reynolds numbers resulting in elastic turbulence. Furthermore, under some conditions, instead of the chaotic turbulence, the result is large-scale waves in the form of cyclic spatial and temporal concentration variations, as has been shown for macromolecular DNA flowing in microfluidic pillar arrays. We here demonstrate how altering the symmetry of the individual pillars can be used to influence the symmetry of these waves. We control the extent of instabilities in viscoelastic flow by leveraging the effects of the symmetry of the pillars on the waves, demonstrating suppressed viscoelastic fluctuations with relevance for transport and sorting applications, or conversely opening up for enhanced viscoelasticity-mediated mixing. The onset of waves, which changes flow resistance, occurs at different Deborah numbers for flow in different directions through the array of triangular pillars, thus breaking the symmetry of the flow resistance along the device, opening up for using the occurrence of the waves to construct a fluidic diode.
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spelling pubmed-106036182023-10-28 Using symmetry to control viscoelastic waves in pillar arrays Beech, Jason P. Ström, Oskar E. Turato, Enrico Tegenfeldt, Jonas O. RSC Adv Chemistry Solutions of macromolecules exhibit viscoelastic properties and unlike Newtonian fluids, they may break time-reversal symmetry at low Reynolds numbers resulting in elastic turbulence. Furthermore, under some conditions, instead of the chaotic turbulence, the result is large-scale waves in the form of cyclic spatial and temporal concentration variations, as has been shown for macromolecular DNA flowing in microfluidic pillar arrays. We here demonstrate how altering the symmetry of the individual pillars can be used to influence the symmetry of these waves. We control the extent of instabilities in viscoelastic flow by leveraging the effects of the symmetry of the pillars on the waves, demonstrating suppressed viscoelastic fluctuations with relevance for transport and sorting applications, or conversely opening up for enhanced viscoelasticity-mediated mixing. The onset of waves, which changes flow resistance, occurs at different Deborah numbers for flow in different directions through the array of triangular pillars, thus breaking the symmetry of the flow resistance along the device, opening up for using the occurrence of the waves to construct a fluidic diode. The Royal Society of Chemistry 2023-10-27 /pmc/articles/PMC10603618/ /pubmed/37901264 http://dx.doi.org/10.1039/d3ra06565k Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by/3.0/
spellingShingle Chemistry
Beech, Jason P.
Ström, Oskar E.
Turato, Enrico
Tegenfeldt, Jonas O.
Using symmetry to control viscoelastic waves in pillar arrays
title Using symmetry to control viscoelastic waves in pillar arrays
title_full Using symmetry to control viscoelastic waves in pillar arrays
title_fullStr Using symmetry to control viscoelastic waves in pillar arrays
title_full_unstemmed Using symmetry to control viscoelastic waves in pillar arrays
title_short Using symmetry to control viscoelastic waves in pillar arrays
title_sort using symmetry to control viscoelastic waves in pillar arrays
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10603618/
https://www.ncbi.nlm.nih.gov/pubmed/37901264
http://dx.doi.org/10.1039/d3ra06565k
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